The editors have included our work in their Editors’ Highlights webpage, which showcases the 50 best papers recently published in this area. You can view the feature on the Editors’ Highlights page (https://www.nature.com/ncomms/editorshighlights) as well as on the journal homepage (https://www.nature.com/ncomms/).
Nanoalignment by Critical Casimir Torques
Gan Wang, Piotr Nowakowski, Nima Farahmand Bafi, Benjamin Midtvedt, Falko Schmidt, Agnese Callegari, Ruggero Verre, Mikael Käll, S. Dietrich, Svyatoslav Kondrat, Giovanni Volpe
Nature Communications, 15, 5086 (2024)
DOI: 10.1038/s41467-024-49220-1
arXiv: 2401.06260
The manipulation of microscopic objects requires precise and controllable forces and torques. Recent advances have led to the use of critical Casimir forces as a powerful tool, which can be finely tuned through the temperature of the environment and the chemical properties of the involved objects. For example, these forces have been used to self-organize ensembles of particles and to counteract stiction caused by Casimir-Liftshitz forces. However, until now, the potential of critical Casimir torques has been largely unexplored. Here, we demonstrate that critical Casimir torques can efficiently control the alignment of microscopic objects on nanopatterned substrates. We show experimentally and corroborate with theoretical calculations and Monte Carlo simulations that circular patterns on a substrate can stabilize the position and orientation of microscopic disks. By making the patterns elliptical, such microdisks can be subject to a torque which flips them upright while simultaneously allowing for more accurate control of the microdisk position. More complex patterns can selectively trap 2D-chiral particles and generate particle motion similar to non-equilibrium Brownian ratchets. These findings provide new opportunities for nanotechnological applications requiring precise positioning and orientation of microscopic objects.
The study, published in Nature Physics and co-written by researchers at the Soft Matter Lab of the Department of Physics at the University of Gothenburg, demonstrate that tunable repulsive critical Casimir forces can be used to counteract stiction, i.e., the tendency of tiny parts of micro- and nanoelectromechanical devices to stick together, which is caused by the Casimir-Lifshitz interaction.
Tunable critical Casimir forces counteract Casimir-Lifshitz attraction
Falko Schmidt, Agnese Callegari, Abdallah Daddi-Moussa-Ider, Battulga Munkhbat, Ruggero Verre, Timur Shegai, Mikael Käll, Hartmut Löwen, Andrea Gambassi and Giovanni Volpe
Nature Physics 19, 271-278 (2023)
arXiv: 2202.10926
doi: 10.1038/s41567-022-01795-6
Casimir forces in quantum electrodynamics emerge between microscopic metallic objects because of the confinement of the vacuum electromagnetic fluctuations occurring even at zero temperature. Their generalization at finite temperature and in material media are referred to as Casimir-Lifshitz forces. These forces are typically attractive, leading to the widespread problem of stiction between the metallic parts of micro- and nanodevices. Recently, repulsive Casimir forces have been experimentally realized but their reliance on specialized materials prevents their dynamic control and thus limits their further applicability. Here, we experimentally demonstrate that repulsive critical Casimir forces, which emerge in a critical binary liquid mixture upon approaching the critical temperature, can be used to actively control microscopic and nanoscopic objects with nanometer precision. We demonstrate this by using critical Casimir forces to prevent the stiction caused by the Casimir-Lifshitz forces. We study a microscopic gold flake above a flat gold-coated substrate immersed in a critical mixture. Far from the critical temperature, stiction occurs because of dominant Casimir-Lifshitz forces. Upon approaching the critical temperature, however, we observe the emergence of repulsive critical Casimir forces that are sufficiently strong to counteract stiction. This experimental demonstration can accelerate the development of micro- and nanodevices by preventing stiction as well as providing active control and precise tunability of the forces acting between their constituent parts.
The two complementary posters focused on the experimental and theoretical/numerical aspects of a system constituted by a micron-sized gold flake suspended in a solution of water-lutidine at critical concentration above a gold-coated substrate. The dynamic of such a system is driven by the interplay of Casimir-Lifshitz forces and critical Casimir forces, which, under convenient circumstances, are the keystone to prevent stiction.
The other two Poster Prizes were awarded to Ariane Soret ( University of Luxembourg, with the poster: Forces Induced by Quantum Mesoscopic Coherent Effects) and Fred Hucht (University of Duisburg-Essen, with the poster: The Square-Lattice Ising Model on the Rectangle).
The Poster Prizes recipients’ names were announced during the closing session on 17 February. Each prize consisted in 100 EUR, which in the case of Agnese and Falko will be shared equally between the two. Andrea Gambassi, who made the announcement on the behalf of the organizers, amusingly mentioned the custom of equally sharing the Nobel Prize.
The Wilhelm and Else Heraeus Foundation is a private institution that supports scientific research and education with an emphasis on physics. It was established in 1963 by Dr. Wilhelm Heinrich Heraeus and his wife Else Heraeus. The Wilhelm and Else Heraeus Foundation is Germany’s most important private institution funding physics.
Casimir-Lifshitz forces vs. Critical Casimir forces: Trapping and releasing of flat metallic particles Falko Schmidt
729. WE-Heraeus Stiftung Seminar on Fluctuation-induced Forces
16 February 2022, 14:50 CET
Casimir forces in quantum electrodynamics emerge between microscopic metallic objects because of the confinement of the vacuum electromagnetic fluctuations occuring even at zero temperature. Their generalization at finite temperature and in material media are referred to as Casimir-Lifshitz forces. These forces are typically attractive, leading to the widespread problem of stiction between the metallic parts of micro- and nanodevices. Recently, repulsive Casimir forces have been experimentally realized but their use of specialized materials stills means that the system can not be controlled dynamically and thus limits further implementation to real-world applications. Here, we experimentally demonstrate that repulsive critical Casimir forces, which emerge in a critical binary liquid mixture upon approaching the critical temperature, can be used to prevent stiction due to Casimir-Lifshitz forces. We show that critical Casimir forces can be dynamically tuned via temperature, eventually overcoming Casimir-Lifshitz attraction. We study a microscopic gold flake above a flat gold-coated substrate immersed in a critical mixture. Far from the critical temperature, stiction occurs because of Casimir-Lifshitz forces. Upon approaching the critical temperature, however, we observe the emergence of repulsive critical Casimir forces that are sufficiently strong to counteract stiction. By removing one of the key limitations to their deployment, this experimental demonstration can accelerate the development of micro- and nanodevices for a broad range of applications.
The article Active Droploids has been featured in a press release of the University of Gothenburg.
The study, published in Nature Communications, examines a special system of colloidal particles and demonstrates a new kind of active matter, which interacts with and modifies its environment. In the long run, the result of the study can be used for drug delivery inside the human body or to perform sensing of environmental pollutants and their clean-up.
Active droploids
Jens Grauer, Falko Schmidt, Jesús Pineda, Benjamin Midtvedt, Hartmut Löwen, Giovanni Volpe & Benno Liebchen
Nat. Commun. 12, 6005 (2021)
doi: 10.1038/s41467-021-26319-3
arXiv: 2109.10677
Active matter comprises self-driven units, such as bacteria and synthetic microswimmers, that can spontaneously form complex patterns and assemble into functional microdevices. These processes are possible thanks to the out-of-equilibrium nature of active-matter systems, fueled by a one-way free-energy flow from the environment into the system. Here, we take the next step in the evolution of active matter by realizing a two-way coupling between active particles and their environment, where active particles act back on the environment giving rise to the formation of superstructures. In experiments and simulations we observe that, under light-illumination, colloidal particles and their near-critical environment create mutually-coupled co-evolving structures. These structures unify in the form of active superstructures featuring a droplet shape and a colloidal engine inducing self-propulsion. We call them active droploids—a portmanteau of droplet and colloids. Our results provide a pathway to create active superstructures through environmental feedback.
The Soft Matter Lab is involved in six presentations at the OSA Biophotonic Congress: Optics in the Life Sciences 2021, topical meeting of Optical Manipulation and its Applications.
Moreover, three of the presentations were selected as finalists for the best student paper in the topical meeting of Optical Manipulation and its Applications.