Nanoalignment by Critical Casimir Torques featured in the Editors’ Highlights of Nature Communications

Artist rendition of a disk-shaped microparticle trapped above a circular uncoated pattern within a thin gold layer coated on a glass surface. (Image by the Authors of the manuscript.)
Our article, entitled Nanoalignment by Critical Casimir Torques, has been selected as a featured article by the editor at Nature Communications. This recognition highlights the significance of our research within the field of applied physics and mathematics.

The editors have included our work in their Editors’ Highlights webpage, which showcases the 50 best papers recently published in this area. You can view the feature on the Editors’ Highlights page (https://www.nature.com/ncomms/editorshighlights) as well as on the journal homepage (https://www.nature.com/ncomms/).

 

Screenshot from the Editors’ Highlights page of Nature Communications, dated 2 July 2024.

Nanoalignment by Critical Casimir Torques published in Nature Communications

Artist rendition of a disk-shaped microparticle trapped above a circular uncoated pattern within a thin gold layer coated on a glass surface. (Image by the Authors of the manuscript.)
Nanoalignment by Critical Casimir Torques
Gan Wang, Piotr Nowakowski, Nima Farahmand Bafi, Benjamin Midtvedt, Falko Schmidt, Agnese Callegari, Ruggero Verre, Mikael Käll, S. Dietrich, Svyatoslav Kondrat, Giovanni Volpe
Nature Communications, 15, 5086 (2024)
DOI: 10.1038/s41467-024-49220-1
arXiv: 2401.06260

The manipulation of microscopic objects requires precise and controllable forces and torques. Recent advances have led to the use of critical Casimir forces as a powerful tool, which can be finely tuned through the temperature of the environment and the chemical properties of the involved objects. For example, these forces have been used to self-organize ensembles of particles and to counteract stiction caused by Casimir-Liftshitz forces. However, until now, the potential of critical Casimir torques has been largely unexplored. Here, we demonstrate that critical Casimir torques can efficiently control the alignment of microscopic objects on nanopatterned substrates. We show experimentally and corroborate with theoretical calculations and Monte Carlo simulations that circular patterns on a substrate can stabilize the position and orientation of microscopic disks. By making the patterns elliptical, such microdisks can be subject to a torque which flips them upright while simultaneously allowing for more accurate control of the microdisk position. More complex patterns can selectively trap 2D-chiral particles and generate particle motion similar to non-equilibrium Brownian ratchets. These findings provide new opportunities for nanotechnological applications requiring precise positioning and orientation of microscopic objects.

Press release on Tunable critical Casimir forces counteract Casimir-Lifshitz attraction

An illustration of microscopic gold flakes on surface. (Image by F. Schmidt.)
The article Tunable critical Casimir forces counteract Casimir-Lifshitz attraction has been featured in the News of the University of Gothenburg (in English and in Swedish), SISSA-International School of Advanced Studies in Trieste, Italy, Heinrich-Heine-Universität Düsseldorf, and Friedrich-Schiller-Universität Jena.

The study, published in Nature Physics and co-written by researchers at the Soft Matter Lab of the Department of Physics at the University of Gothenburg, demonstrate that tunable repulsive critical Casimir forces can be used to counteract stiction, i.e., the tendency of tiny parts of micro- and nanoelectromechanical devices to stick together, which is caused by the Casimir-Lifshitz interaction.

The study is featured also in Phys.org, NanoWerk.

Here the links to the press releases:
Casimir vs Casimir – using opposing forces to improve nanotechnology (GU, English)
https://www.gu.se/nyheter/casimir-vs-casimir-klaschande-krafter-kan-forbattra-nanotekniken (GU, Swedish)
Casimir vs Casimir – usare forze opposte per migliorare le nanotecnologie (SISSA, Italian)
Casimir vs Casimir – using opposing forces to improve nanotechnology (SISSA, English)
Nano-Bauteile clever voneinander lösen (Heinrich-Heine-Universität Düsseldorf)
Clever method for separating nano-components (Friedrich-Schiller-Universität Jena)
Clever method for separating nano-components (Phys.org)
Clever method for separating nano-components (NanoWerk)

Tunable critical Casimir forces counteract Casimir-Lifshitz attraction published in Nature Physics

Gold flake suspended over a functionalized gold-coated substrate. (Image by F. Schmidt.)
Tunable critical Casimir forces counteract Casimir-Lifshitz attraction
Falko Schmidt, Agnese Callegari, Abdallah Daddi-Moussa-Ider, Battulga Munkhbat, Ruggero Verre, Timur Shegai, Mikael Käll, Hartmut Löwen, Andrea Gambassi and Giovanni Volpe
Nature Physics 19, 271-278 (2023)
arXiv: 2202.10926
doi: 10.1038/s41567-022-01795-6

Casimir forces in quantum electrodynamics emerge between microscopic metallic objects because of the confinement of the vacuum electromagnetic fluctuations occurring even at zero temperature. Their generalization at finite temperature and in material media are referred to as Casimir-Lifshitz forces. These forces are typically attractive, leading to the widespread problem of stiction between the metallic parts of micro- and nanodevices. Recently, repulsive Casimir forces have been experimentally realized but their reliance on specialized materials prevents their dynamic control and thus limits their further applicability. Here, we experimentally demonstrate that repulsive critical Casimir forces, which emerge in a critical binary liquid mixture upon approaching the critical temperature, can be used to actively control microscopic and nanoscopic objects with nanometer precision. We demonstrate this by using critical Casimir forces to prevent the stiction caused by the Casimir-Lifshitz forces. We study a microscopic gold flake above a flat gold-coated substrate immersed in a critical mixture. Far from the critical temperature, stiction occurs because of dominant Casimir-Lifshitz forces. Upon approaching the critical temperature, however, we observe the emergence of repulsive critical Casimir forces that are sufficiently strong to counteract stiction. This experimental demonstration can accelerate the development of micro- and nanodevices by preventing stiction as well as providing active control and precise tunability of the forces acting between their constituent parts.

Flash Talk by F. Schmidt at 729. WE Heraeus Seminar on Fluctuation Induced Forces, Online, 16 February 2022

Title slide of the presentation. (Image by F. Schmidt.)
Casimir-Lifshitz forces vs. Critical Casimir forces: Trapping and releasing of flat metallic particles
Falko Schmidt
729. WE-Heraeus Stiftung Seminar on Fluctuation-induced Forces
16 February 2022, 14:50 CET

Casimir forces in quantum electrodynamics emerge between microscopic metallic objects because of the confinement of the vacuum electromagnetic fluctuations occuring even at zero temperature. Their generalization at finite temperature and in material media are referred to as Casimir-Lifshitz forces. These forces are typically attractive, leading to the widespread problem of stiction between the metallic parts of micro- and nanodevices. Recently, repulsive Casimir forces have been experimentally realized but their use of specialized materials stills means that the system can not be controlled dynamically and thus limits further implementation to real-world applications. Here, we experimentally demonstrate that repulsive critical Casimir forces, which emerge in a critical binary liquid mixture upon approaching the critical temperature, can be used to prevent stiction due to Casimir-Lifshitz forces. We show that critical Casimir forces can be dynamically tuned via temperature, eventually overcoming Casimir-Lifshitz attraction. We study a microscopic gold flake above a flat gold-coated substrate immersed in a critical mixture. Far from the critical temperature, stiction occurs because of Casimir-Lifshitz forces. Upon approaching the critical temperature, however, we observe the emergence of repulsive critical Casimir forces that are sufficiently strong to counteract stiction. By removing one of the key limitations to their deployment, this experimental demonstration can accelerate the development of micro- and nanodevices for a broad range of applications.

Microscopic Metavehicles Powered and Steered by Embedded Optical Metasurfaces published in Nature Nanotechnology

Metavehicles.
Microscopic Metavehicles Powered and Steered by Embedded Optical Metasurfaces
Daniel Andrén, Denis G. Baranov, Steven Jones, Giovanni Volpe, Ruggero Verre, Mikael Käll
Nat. Nanotechnol. (2021)
doi: 10.1038/s41565-021-00941-0
arXiv: 2012.10205

Nanostructured dielectric metasurfaces offer unprecedented opportunities to manipulate light by imprinting an arbitrary phase gradient on an impinging wavefront. This has resulted in the realization of a range of flat analogues to classical optical components, such as lenses, waveplates and axicons. However, the change in linear and angular optical momentum associated with phase manipulation also results in previously unexploited forces and torques that act on the metasurface itself. Here we show that these optomechanical effects can be utilized to construct optical metavehicles – microscopic particles that can travel long distances under low-intensity plane-wave illumination while being steered by the polarization of the incident light. We demonstrate movement in complex patterns, self-correcting motion and an application as transport vehicles for microscopic cargoes, which include unicellular organisms. The abundance of possible optical metasurfaces attests to the prospect of developing a wide variety of metavehicles with specialized functional behaviours.